Palmer Group @ Edinburgh::
Satellite Observations of Tropospheric Composition
Introduction
Space-borne measurements of the composition of Earth's lower
atmosphere are relatively new. We, as a community, are just
beginning to make full use of these data to learn about Earth's
atmosphere. Currenty there are several satellite instruments
orbiting the Earth (most of which are in the A-train) that can
measure
tropospheric O3 and many of its photochemical precursors
(e.g., NO2, formaldehyde), CO, CO2,
CH4,
and aerosol optical properties. The biggest challenge facing the
chemistry-climate community is how to best use these data. Below
is a list of some projects we are currently involved with.
The A-train satellite constellation
(flanked by Aura and Aqua) plus OCO
General Areas of Current Research
GOME, SCIAMACHY and OMI
In an ongoing collaboration with
Kelly Chance
and his group (Harvard-Smithsonian Center for Astrophysics) and
with Folkert Wittrock (University of Bremen) we
analyze column observations of formaldehyde, NO2 and
tropospheric O3 from the Global Ozone Monitoring
Experiment (GOME), SCIAMACHY and the Ozone Monitoring Experiment
(OMI) [1-9]. Our collaborative work is the first to fully exploit
column observations of formaldehyde as constraints on biogenic VOC
emissions. We are also assessing CO2 column measurements
from SCIAMACHY.
TES
The Aura spacecraft,
launched in July 2004, is the first mission
dedicated to understanding atmospheric composition. The Tropospheric
Emission Spectrometer (TES) is a key instrument aboard Aura that
observes a range of tropospheric gases. In collaboration with the
TES group at JPL we are investigating the potential of these data,
together with other instruments aboard Aura, to improve
understanding of biomass burning emissions and how they affect
tropospheric ozone.
OCO and GOSAT
The Orbiting Carbon
Observatory and the Greenhouse gases Observing
SATellite, both due for launch in 2008, are designed to measure
column CO2 to 1ppm precision. Liang Feng is developing
an assimilation framework to use these data for source/sink
estimation.
MODIS and MISR
The MODIS and
MISR instruments
provide a wide range of environmental information, including
aerosol optical properties, cloud optical properties, ocean color
(a proxy for marine biomass [10]), sea-surface temperature, and land
cover characteristics. Claire Bulgin has been using the GRAPE aerosol and cloud
dataset to investigate the Twomey indirect effect. We are
also preparing assimilation experiments to test model descriptions
of aerosol processes.
[1]
Palmer, P. I., et al, J. Geophys. Res.., doi:10.1029/2005JD006689,
2006. (PDF)
[2]
Liu, X., et al, J. Geophys. Res.., doi:10.1029/2005JD006564,
2006.
(PDF)
[3]
Shim, C., et al, J. Geophys. Res.,
doi:10.1029/2004JD005629, 2005.
(PDF)
[4]
Palmer, P. I., et al, J. Geophys. Res.,
doi:10.1029/2002JD002153, 2003.
(PDF)
[5]
Abbot, D. S., et al,
Geophys. Res. Lett. doi:10.1029/2003GL017336, 2003.
(PDF).
Journal cover.
[6]
Martin, R. V., et al,
J. Geophys. Res., doi: 10.1029/2003JD003453, 2003.
(PDF)
[7]
Martin, R. V., et al, J. Geophys. Res.,
10.1029/2001JD001027, 2002. (PDF)
[8]
Palmer, P. I., et al, J. Geophys. Res., 106, 14539-14550,
2001. (PDF)
[9]
Chance, K., et al, Geophys. Res. Lett, 27, 3461-3464, 2000.
(PDF)
[10] Palmer, P. I. and S. Shaw, Geophys. Res.
Lett., doi:10.1029/2005GL022592, 2005.
(PDF).
[Isoprene Ocean Flux Data].